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Beilstein J. Org. Chem. 2014, 10, 936–947, doi:10.3762/bjoc.10.92
Graphical Abstract
Scheme 1: Chemical structures of RB, EDB and TA.
Scheme 2: Type II PIS mechanisms. PS: photosensitizer; 1,3PS*: singlet and triplet PS excited states; PS•+: o...
Figure 1: Evolution of RB concentration as a function of irradiation time (λ = 532 nm, 9 mW·cm−3); insert: ab...
Scheme 3: Photocatalytic behavior occurring in three component PIS. PS: photosensitizer; 1,3PS*: singlet and ...
Figure 2: Evolution of [RB](t) in the photocyclic system RB/TA/EDB as a function of irradiation time (λ = 532...
Scheme 4: Thermodynamics of an oxidative three components PCIS, a) ground state reaction (), b) excited state...
Scheme 5: General photocatalytic cycle occurring in three components photocyclic systems. Two cycles are in c...
Figure 3: Mechanistic description of photocyclic system involved in the RB/TA/EDB system. The rate constants ...
Figure 4: Evolution of RB, RB•+, TA, and TA•− concentration with time for RB/TA system.
Figure 5: Evolution of RB, TA and EDB concentrations in the photocyclic system. The logarithm of oxidative an...
Figure 6: Evolution of radical concentrations TA•− and EDB•+ together with [RB] in photocatalytic system.